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Leistungen
A set of photocathode membrane assemblies with included protection layers and/or HER electrocatalysts, with at least one asssembly that achieves (or has a concrete action plan to achieve) a water splitting photocurrent of 8.2 mA/cm2 under standard solar illumination.
Visual identity, project website and social media accountsVisual identity (including a logo) and website will be designed to ensure brand consistency, recognition and visibility of Sun-To-X. Social media accounts (Twitter and LinkedIn) will be created and fed through for the project duration to communicate about the project and disseminate its key results.
Report on preliminary testsReport on the preliminary tests before the commissioning/operation of the demonstrator, assuring that the engineering and safety specifications are met.
Demonstration of prototype 100 cm2 PEM-PEC cellA medium size upscaled PEM-PEC device will be up and running. The demo PEM-PEC cell will be developed using state of the art materials. This demo unit will be used as guiding example for the final upscaling step that will be performed in WP5.
Demonstration of large area (100 cm2) prototype membrane photoanode assembly suitable for integration in the large area prototype deviceSet of 5 photoanode assemblies, fabricated based on the results in D1.3, with a size of at least 100 cm2 per assembly.
A catalytic system will be developped and its potential in the conversion of model substrates representatives of the chemical linkages present in waste plastics will be demonstrated This deliverable hence include the reduction of aliphatic and aromatic esters as well as organic carbonates using HydroSil as the reductant
Intermediate Advisory Board recommendations reportReport summarising the advisory board recommendations after the first meeting The meeting should have been attended by all advisory board members and the coordinator Relevant feedback should be discussed between the coordinator and SuntoX participants Where relevant a clear plan for implementing advice should be made
Final report on Dissemination & Communication activitiesThis report will give an overview of the Dissemination and Communication actions implemented during the 42 months project and how they performed with the respect to the target set in the Dissemination and Communication Plan.
Final Advisory Board recommendations reportReport summarising the advisory board recommendations after the second meeting. The meeting should have been attended by all advisory board members and the coordinator. Relevant feedback should be discussed between the coordinator and Sun-to-X participants (EPFL / ENGIE). Where relevant, a clear plan for implementing advice in the demonstrator stage should be made.
Demonstration of the production of n-hexane by catalytic depolymerization of waste polycaprolactone using HydroSilThe conversion of polycaprolactone, a polyester, to n-hexane will be demonstrated using HydroSil as the reductant and the catalytic system elaborated by CEA. The products will be isolated to recover n-hexane and the silicon oxide (siloxane).
Data Management PlanDescription of the data management plan for the project
Report on the activities of collaboration with IC5Report summarising the actions during the project with Mission Innovation IC5- contributions to their roadmap, demonstration activites, synergies / interactions with other IC5 projects
Social factors hindering the marketAnalysis of the potential social impacts of this technology, including acceptance and controversy management.
Guidelines generated from the validated multi-physics model of the PEC deviceModel should give reasonable predictions of photocurrent same order of magnitude after validation Strategies to improve performance by considering for example efficiency of light absorption and current collection should be presented
Developed techno-economic model of the deviceTechnoeconomic model containing all relevant costs. A breakdown of costs should be clearly shown to identify strategies for future cost reduction. A comparison of the cost between vapour and liquid should be shown.
Report on the performance evaluation of the prototype in realistic conditionsReport summarising the relationship of photoelectrode surface area and performance of the most promising material combinations. This deliverable includes outdoor measurements.
Veröffentlichungen
Autoren:
Gideon Segev; Jakob Kibsgaard; Christopher Hahn; Zhichuan J Xu; Wen-Hui (Sophia) Cheng; Todd G Deutsch; Chengxiang Xiang; Jenny Z Zhang; Leif Hammarström; Daniel G Nocera; Adam Z Weber; Peter Agbo; Takashi Hisatomi; Frank E Osterloh; Kazunari Domen; Fatwa F Abdi; Sophia Haussener; Daniel J Miller; Shane Ardo; Paul C McIntyre; Thomas Hannappel; Shu Hu; Harry Atwater; John M Gregoire; Mehmed Z Erte
Veröffentlicht in:
Journal of Physics D: Applied Physics, 2022, Seite(n) Volume 55 Article 323003, ISSN 0022-3727
Herausgeber:
Institute of Physics Publishing
DOI:
10.1088/1361-6463/ac6f97
Autoren:
Caroline Keller Yassine Djezzar, Jingxian Wang, Saravanan Karuppiah, Gérard Lapertot, Cédric Haon, and Pascale Chenevier
Veröffentlicht in:
Nanomaterials, Ausgabe 28 July 2022, 2022, Seite(n) 2601, ISSN 2079-4991
Herausgeber:
MDPI
DOI:
10.3390/nano12152601
Autoren:
Marie Kobylarski, Liam J. Donnelly, Jean-Claude Berthet and Thibault Cantat
Veröffentlicht in:
Green Chemistry, Ausgabe 27 Aug 2022, 2022, Seite(n) 6810-6815, ISSN 1463-9262
Herausgeber:
Royal Society of Chemistry
DOI:
10.1039/d2gc02186b
Autoren:
Marina Caretti, Linda Lazouni, Meng Xia, Rebekah A. Wells, Simon Nussbaum, Dan Ren, Michael Grätzel, and Kevin Sivula*
Veröffentlicht in:
ACS Energy Letters, 2022, ISSN 2380-8195
Herausgeber:
American Chemical Society
DOI:
10.1021/acsenergylett.2c00474
Autoren:
Jingxian Wang, Caroline Keller, Marc Dietrich, Paul E. Olli, Pascal Gentile, Stéphanie Pouget, Hanako Okuno, Mohamed Boutghatin, Yan Pennec, Valérie Reita, Duc N. Nguyen, Hannah Johnson, Adina Morozan, Vincent Artero and Pascale Chenevier
Veröffentlicht in:
Sustainable Energy & Fuels, Ausgabe 23 August 2023, 2023, Seite(n) 4864-4876, ISSN 2398-4902
Herausgeber:
Royal Society of Chemistry
DOI:
10.1039/d3se00408b
Autoren:
Marina Caretti, Elizaveta Mensi, Raluca-Ana Kessler, Linda Lazouni, Benjamin Goldman, Loï Carbone, Simon Nussbaum, Rebekah A. Wells, Hannah Johnson, Emeline Rideau, Jun-ho Yum, Kevin Sivula
Veröffentlicht in:
Advanced Materials, Ausgabe 28 November 2022, 2022, Seite(n) 2208740, ISSN 1521-4095
Herausgeber:
Wiley
DOI:
10.1002/adma.202208740
Autoren:
Alexandre Cattry, Hannah Johnson, Despoina Chatzikiriakou, and Sophia Haussener
Veröffentlicht in:
Energy & Fuels, Ausgabe 4 July 2024, 2024, Seite(n) 11363-12282, ISSN 0887-0624
Herausgeber:
American Chemical Society
DOI:
10.1021/acs.energyfuels.4c00936
Autoren:
Dr. Liam J. Donnelly, Dr. Jean-Claude Berthet, Dr. Thibault Cantat
Veröffentlicht in:
Angewandte Chemie, Ausgabe 18 May 2022, 2022, Seite(n) e202206170, ISSN 1433-7851
Herausgeber:
John Wiley & Sons Ltd.
DOI:
10.1002/anie.202206170
Autoren:
Jean-Claude BERTHET, Thibault CANTAT ,Cyril THEULIER
Veröffentlicht in:
2024
Herausgeber:
ChemRxiv
DOI:
10.26434/chemrxiv-2024-m4x02
Autoren:
Hannah Johnson
Veröffentlicht in:
Innovation News Network, Ausgabe 19th April 2023, 2023
Herausgeber:
Innovation News Network
Autoren:
Mary Hanhoun, Jonas Pigeon, Julie Clavreul, Laurent Baraton, Hannah Johnson
Veröffentlicht in:
FISITA Conference Proceedings, Ausgabe 12th September 2023, 2023
Herausgeber:
FISITA
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