New Directions in Sustainable Catalysis by Metal Complexes

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Les liens vers les livrables et les publications des projets du 7e PC, ainsi que les liens vers certains types de résultats spécifiques tels que les jeux de données et les logiciels, sont récupérés dynamiquement sur OpenAIRE .

Publications

Acceptorless dehydrogenative synthesis of primary amides from alcohols and ammonia

Auteurs: Jie Luo, Quan-Quan Zhou, Michael Montag, Yehoshoa Ben-David and David Milstein
Publié dans: Chemical Science, 2022, ISSN 2041-6520
Éditeur: Royal Society of Chemistry
DOI: 10.1039/d1sc07102e

Highly efficient additive-free dehydrogenation of neat formic acid

Auteurs: Sayan Kar, Michael Rauch, Gregory Leitus, Yehoshoa Ben-David and David Milstein
Publié dans: Nature Catalysis, 2021, ISSN 2520-1158
Éditeur: Nature Research (United Kingdom)
DOI: 10.1038/s41929-021-00575-4

Formation of thioesters by dehydrogenative coupling of thiols and alcohols with H(2)evolution

Auteurs: Jie Luo, Michael Rauch, Liat Avram, Yael Diskin-Posner, Guy Shmul, Yehoshoa Ben-David and David Milstein
Publié dans: Nature Catalysis, 2020, ISSN 2520-1158
Éditeur: Nature Publishing Group
DOI: 10.1038/s41929-020-00514-9

Dehydrogenative Cross-Coupling of Primary Alcohols To Form Cross-Esters Catalyzed by a Manganese Pincer Complex

Auteurs: Uttam Kumar Das, Yehoshoa Ben-David, Gregory Leitus, Yael Diskin-Posner, David Milstein
Publié dans: ACS Catalysis, Numéro 9/1, 2018, Page(s) 479-484, ISSN 2155-5435
Éditeur: American Chemical Society
DOI: 10.1021/acscatal.8b04585

Direct Synthesis of Amides by Acceptorless Dehydrogenative Coupling of Benzyl Alcohols and Ammonia Catalyzed by a Manganese Pincer Complex: Unexpected Crucial Role of Base: Unexpected Crucial Role of Base.

Auteurs: Prosenjit Daw, Amit Kumar, Noel Angel Espinosa-Jalapa, Yehoshoa Ben-David, and David Milstein
Publié dans: J. Am. Chem. Soc., 2019, ISSN 0002-7863
Éditeur: American Chemical Society
DOI: 10.1021/jacs.9b05261

Near-Ambient-Temperature Dehydrogenative Synthesis of the Amide Bond: Mechanistic Insight and Applications: Mechanistic Insight and Applications: Mechanistic Insight and Applications

Auteurs: Sayan Kar; Yinjun Xie; Quan Quan Zhou; Yael Diskin-Posner; Yehoshoa Ben-David; David Milstein
Publié dans: ACS catalysis, 2021, ISSN 2155-5435
Éditeur: American Chemical Society
DOI: 10.1021/acscatal.1c00728

Efficient Base-Free Aqueous Reforming of Methanol Homogeneously Catalyzed by Ruthenium Exhibiting a Remarkable Acceleration by Added Catalytic Thiol.

Auteurs: Jie Luo; Sayan Kar; Michael Rauch; Michael Montag; Yehoshoa Ben-David; David Milstein
Publié dans: Journal of the American Chemical Society, Numéro 5, 2021, ISSN 0002-7863
Éditeur: American Chemical Society
DOI: 10.1021/jacs.1c09007

Mechanistic Investigations of Ruthenium Catalyzed Dehydrogenative Thioester Synthesis and Thioester Hydrogenation

Auteurs: Michael Rauch, Jie Luo, Liat Avram, Yehoshoa Ben-David and David Milstein
Publié dans: ACS Catalysis, 2021, ISSN 2155-5435
Éditeur: American Chemical Society
DOI: 10.1021/acscatal.1c00418

Oxidation of Alkenes by Water with H 2 Liberation

Auteurs: Shan Tang, Yehoshoa Ben-David, David Milstein
Publié dans: Journal of the American Chemical Society, Numéro 142/13, 2020, Page(s) 5980-5984, ISSN 0002-7863
Éditeur: American Chemical Society
DOI: 10.1021/jacs.0c01592

Pd Catalyzed, Acid Accelerated, Rechargeable, Liquid Organic Hydrogen Carrier System Based on Methylpyridines/Methylpiperidines

Auteurs: Yinjun Xie and David Milstein
Publié dans: ACS Applied Energy Materials, 2019, ISSN 2574-0962
Éditeur: American Chemical society
DOI: 10.1021/acsaem.9b00523

Homogeneous Catalysis for Sustainable Energy: Hydrogen and Methanol Economies, Fuels from Biomass, and Related Topics

Auteurs: Amit Kumar, Prosenjit Daw and David Milstein
Publié dans: Chemical Reviews, 2021, ISSN 0009-2665
Éditeur: American Chemical Society
DOI: 10.1021/acs.chemrev.1c00412

Dehydrogenative ester synthesis from enol ethers and water with a ruthenium complex catalyzing two reactions in synergy

Auteurs: Sayan Kar; Jie Luo; Michael Rauch; Yael Diskin-Posner; Yehoshoa Ben-David; David Milstein
Publié dans: Crossref, Numéro 1, 2022, ISSN 1463-9262
Éditeur: Royal Society of Chemistry
DOI: 10.1039/d1gc04574a

Formamides as Isocyanate Surrogates: A Mechanistically Driven Approach to the Development of Atom-Efficient, Selective Catalytic Syntheses of Ureas, Carbamates, and Heterocycles: A Mechanistically Driven Approach to the Development of Atom-Efficient, Selective Catalytic Syntheses of Ureas, Carbamates, and Heterocycles

Auteurs: Jeffrey Bruffaerts, Niklas Von Wolff, Yael Diskin Posner, Yehoshoa Ben-David and David Milstein
Publié dans: Journal of the American Chemical Society, 2019, ISSN 0002-7863
Éditeur: American Chemical Society
DOI: 10.1021/jacs.9b08942

A Reversible Liquid Organic Hydrogen Carrier System Based on Methanol-Ethylenediamine and Ethylene Urea

Auteurs: Yinjun Xie, Peng Hu, Yehoshoa Ben-David and David Milstein
Publié dans: Angewandte Chemie - International Edition, 2019, ISSN 1433-7851
Éditeur: John Wiley & Sons Ltd.
DOI: 10.1002/anie.201901695

Heterogeneously catalyzed selective hydrogenation of amides to alcohols and amines (No embargo, Accepted version

Auteurs: Yinjun Xie, Peng Hu, Tatyana Bendikov and David Milstein
Publié dans: Catalysis Science and Technology, 2018, ISSN 2044-4753
Éditeur: Royal Society of Chemistry
DOI: 10.1039/c8cy00112j

Template catalysis by manganese pincer complexes: oxa- and aza-Michael additions to unsaturated nitriles† †Electronic supplementary information (ESI) available. See DOI: 10.1039/c9sc03269j

Auteurs: Tang, Shan; Milstein, David
Publié dans: Chemical Science, Numéro 1, 2019, ISSN 2041-6520
Éditeur: Royal Society of Chemistry
DOI: 10.1039/c9sc03269j

Metal–Ligand Cooperation Facilitates Bond Activation and Catalytic Hydrogenation with Zinc Pincer Complexes

Auteurs: Michael Rauch, Sayan Kar, Amit Kumar, Liat Avram, Linda J. W. Shimon, David Milstein
Publié dans: Journal of the American Chemical Society, Numéro 142/34, 2020, Page(s) 14513-14521, ISSN 0002-7863
Éditeur: American Chemical Society
DOI: 10.1021/jacs.0c05500

Pyridine-Based PCP-Ruthenium Complexes: Unusual Structures and Metal–Ligand Cooperation

Auteurs: Pyridine-Based PCP-Ruthenium Complexes: Unusual Structures and Metal–Ligand Cooperation Shan Tang, Niklas von Wolff, Yael Diskin-Posner, Gregory Leitus, Yehoshoa Ben-David, and David Milstein
Publié dans: J. Am. Chem. Soc., 2019, ISSN 0002-7863
Éditeur: American Chemical Society
DOI: 10.1021/jacs.9b02669

Synthesis of oxalamides by acceptorless dehydrogenative coupling of ethylene glycol and amines and the reverse hydrogenation catalyzed by ruthenium

Auteurs: You-Quan Zou, Quan-Quan Zhou, Yael Diskin-Posner, Yehoshoa Ben-David, David Milstein
Publié dans: Chemical Science, Numéro 11/27, 2020, Page(s) 7188-7193, ISSN 2041-6520
Éditeur: Royal Society of Chemistry
DOI: 10.1039/d0sc02065f

Hydrogenative Depolymerization of Nylons

Auteurs: Amit Kumar, Niklas von Wolff, Michael Rauch, You-Quan Zou, Guy Shmul, Yehoshoa Ben-David, Gregory Leitus, Liat Avram, David Milstein
Publié dans: Journal of the American Chemical Society, Numéro 142/33, 2020, Page(s) 14267-14275, ISSN 0002-7863
Éditeur: American Chemical Society
DOI: 10.1021/jacs.0c05675

Selective Room-Temperature Hydrogenation of Amides to Amines and Alcohols Catalyzed by a Ruthenium Pincer Complex and Mechanistic Insight

Auteurs: Sayan Kar, Michael Rauch, Amit Kumar, Gregory Leitus, Yehoshoa Ben-David, David Milstein
Publié dans: ACS Catalysis, Numéro 10/10, 2020, Page(s) 5511-5515, ISSN 2155-5435
Éditeur: American Chemical Society
DOI: 10.1021/acscatal.0c01406

Manganese-Pincer-Catalyzed Nitrile Hydration, α‑Deuteration, and α‑Deuterated Amide Formation via Metal Ligand Cooperation

Auteurs: Quan-Quan Zhou, You-Quan Zou, Sayan Kar, Yael Diskin-Posner, Yehoshoa Ben-David and David Milstein
Publié dans: ACS Catalysis, 2021, ISSN 2155-5435
Éditeur: American Chemical Society

Direct Synthesis of Symmetrical Azines from Alcohols and Hydrazine Catalyzed by a Ruthenium Pincer Complex: Effect of Hydrogen Bonding

Auteurs: Jonathan O. Bauer, Gregory Leitus, Yehoshoa Ben-David, David Milstein
Publié dans: ACS Catalysis, Numéro 6/12, 2016, Page(s) 8415-8419, ISSN 2155-5435
Éditeur: American Chemical Society
DOI: 10.1021/acscatal.6b02946

Hydrogenation and Hydrosilylation of Nitrous Oxide Homogeneously Catalyzed by a Metal Complex

Auteurs: Rong Zeng, Moran Feller, Yehoshoa Ben-David, David Milstein
Publié dans: Journal of the American Chemical Society, Numéro 139/16, 2017, Page(s) 5720-5723, ISSN 0002-7863
Éditeur: American Chemical Society
DOI: 10.1021/jacs.7b02124

The Ferraquinone–Ferrahydroquinone Couple: Combining Quinonic and Metal-Based Reactivity

Auteurs: Alexander Dauth, Urs Gellrich, Yael Diskin-Posner, Yehoshoa Ben-David, David Milstein
Publié dans: Journal of the American Chemical Society, Numéro 139/7, 2017, Page(s) 2799-2807, ISSN 0002-7863
Éditeur: American Chemical Society
DOI: 10.1021/jacs.6b13050

Highly Selective, Efficient Deoxygenative Hydrogenation of Amides Catalyzed by a Manganese Pincer Complex via Metal–Ligand Cooperation

Auteurs: You-Quan Zou, Subrata Chakraborty, Alexander Nerush, Dror Oren, Yael Diskin-Posner, Yehoshoa Ben-David, David Milstein
Publié dans: ACS Catalysis, Numéro 8/9, 2018, Page(s) 8014-8019, ISSN 2155-5435
Éditeur: American Chemical Society
DOI: 10.1021/acscatal.8b02902

Homogeneous Catalysis by Cobalt and Manganese Pincer Complexes

Auteurs: Arup Mukherjee, David Milstein
Publié dans: ACS Catalysis, Numéro 8/12, 2018, Page(s) 11435-11469, ISSN 2155-5435
Éditeur: American Chemical Society
DOI: 10.1021/acscatal.8b02869

Metal–Ligand Cooperation as Key in Formation of Dearomatized Ni II –H Pincer Complexes and in Their Reactivity toward CO and CO 2

Auteurs: Dror Oren, Yael Diskin-Posner, Liat Avram, Moran Feller, David Milstein
Publié dans: Organometallics, Numéro 37/14, 2018, Page(s) 2217-2221, ISSN 0276-7333
Éditeur: American Chemical Society
DOI: 10.1021/acs.organomet.8b00160

N-Substituted Hydrazones by Manganese-Catalyzed Coupling of Alcohols with Hydrazine: Borrowing Hydrogen and Acceptorless Dehydrogenation in One System

Auteurs: Uttam Kumar Das, Yehoshoa Ben-David, Yael Diskin-Posner, David Milstein
Publié dans: Angewandte Chemie International Edition, Numéro 57/8, 2018, Page(s) 2179-2182, ISSN 1433-7851
Éditeur: John Wiley & Sons Ltd.
DOI: 10.1002/anie.201712593

Direct Synthesis of Benzimidazoles by Dehydrogenative Coupling of Aromatic Diamines and Alcohols Catalyzed by Cobalt

Auteurs: Prosenjit Daw, Yehoshoa Ben-David, David Milstein
Publié dans: ACS Catalysis, Numéro 7/11, 2017, Page(s) 7456-7460, ISSN 2155-5435
Éditeur: American Chemical Society
DOI: 10.1021/acscatal.7b02777

CO 2 activation by metal − ligand-cooperation mediated by iridium pincer complexes

Auteurs: Moran Feller, Eyal Ben-Ari, Yael Diskin-Posner, David Milstein
Publié dans: Journal of Coordination Chemistry, Numéro 71/11-13, 2018, Page(s) 1679-1689, ISSN 0095-8972
Éditeur: Gordon and Breach Science Publishers
DOI: 10.1080/00958972.2018.1475662

Formal oxidative addition of a C–H bond by a 16e iridium( i ) complex involves metal–ligand cooperation

Auteurs: Amit Kumar, Moran Feller, Yehoshoa Ben-David, Yael Diskin-Posner, David Milstein
Publié dans: Chemical Communications, Numéro 54/42, 2018, Page(s) 5365-5368, ISSN 1359-7345
Éditeur: Royal Society of Chemistry
DOI: 10.1039/c8cc01885e

Imidazole synthesis by transition metal free, base-mediated deaminative coupling of benzylamines and nitriles

Auteurs: Uttam Kumar Das, Linda J. W. Shimon, David Milstein
Publié dans: Chemical Communications, Numéro 53/98, 2017, Page(s) 13133-13136, ISSN 1359-7345
Éditeur: Royal Society of Chemistry
DOI: 10.1039/c7cc08322j

Manganese Catalyzed α-Olefination of Nitriles by Primary Alcohols

Auteurs: Subrata Chakraborty, Uttam Kumar Das, Yehoshoa Ben-David, David Milstein
Publié dans: Journal of the American Chemical Society, Numéro 139/34, 2017, Page(s) 11710-11713, ISSN 0002-7863
Éditeur: American Chemical Society
DOI: 10.1021/jacs.7b06993

Manganese-Catalyzed α-Alkylation of Ketones, Esters, and Amides Using Alcohols

Auteurs: Subrata Chakraborty, Prosenjit Daw, Yehoshoa Ben David, David Milstein
Publié dans: ACS Catalysis, Numéro 8/11, 2018, Page(s) 10300-10305, ISSN 2155-5435
Éditeur: American Chemical Society
DOI: 10.1021/acscatal.8b03720

Selective Hydrogenation of Cyclic Imides to Diols and Amines and Its Application in the Development of a Liquid Organic Hydrogen Carrier

Auteurs: Amit Kumar, Trevor Janes, Noel Angel Espinosa-Jalapa, David Milstein
Publié dans: Journal of the American Chemical Society, Numéro 140/24, 2018, Page(s) 7453-7457, ISSN 0002-7863
Éditeur: American Chemical Society
DOI: 10.1021/jacs.8b04581

Synthesis of Cyclic Imides by Acceptorless Dehydrogenative Coupling of Diols and Amines Catalyzed by a Manganese Pincer Complex

Auteurs: Noel Angel Espinosa-Jalapa, Amit Kumar, Gregory Leitus, Yael Diskin-Posner, David Milstein
Publié dans: Journal of the American Chemical Society, Numéro 139/34, 2017, Page(s) 11722-11725, ISSN 0002-7863
Éditeur: American Chemical Society
DOI: 10.1021/jacs.7b08341

Direct Synthesis of Amides by Dehydrogenative Coupling of Amines with either Alcohols or Esters: Manganese Pincer Complex as Catalyst

Auteurs: Amit Kumar, Noel Angel Espinosa-Jalapa, Gregory Leitus, Yael Diskin-Posner, Liat Avram, David Milstein
Publié dans: Angewandte Chemie International Edition, Numéro 56/47, 2017, Page(s) 14992-14996, ISSN 1433-7851
Éditeur: John Wiley & Sons Ltd.
DOI: 10.1002/anie.201709180

Manganese Catalyzed Hydrogenation of Organic Carbonates to Methanol and Alcohols

Auteurs: Amit Kumar, Trevor Janes, Noel Angel Espinosa-Jalapa, David Milstein
Publié dans: Angewandte Chemie International Edition, Numéro 57/37, 2018, Page(s) 12076-12080, ISSN 1433-7851
Éditeur: John Wiley & Sons Ltd.
DOI: 10.1002/anie.201806289

Acceptorless Dehydrogenative Coupling Using Ammonia: Direct Synthesis of N-Heteroaromatics from Diols Catalyzed by Ruthenium

Auteurs: Prosenjit Daw, Yehoshoa Ben-David, David Milstein
Publié dans: Journal of the American Chemical Society, Numéro 140/38, 2018, Page(s) 11931-11934, ISSN 0002-7863
Éditeur: American Chemical Society
DOI: 10.1021/jacs.8b08385

Direct Conversion of Alcohols into Alkenes by Dehydrogenative Coupling with Hydrazine/Hydrazone Catalyzed by Manganese

Auteurs: Uttam Kumar Das, Subrata Chakraborty, Yael Diskin-Posner, David Milstein
Publié dans: Angewandte Chemie International Edition, Numéro 57/41, 2018, Page(s) 13444-13448, ISSN 1433-7851
Éditeur: John Wiley & Sons Ltd.
DOI: 10.1002/anie.201807881

Synthesis of Pyrazines and Quinoxalines via Acceptorless Dehydrogenative Coupling Routes Catalyzed by Manganese Pincer Complexes

Auteurs: Prosenjit Daw, Amit Kumar, Noel Angel Espinosa-Jalapa, Yael Diskin-Posner, Yehoshoa Ben-David, David Milstein
Publié dans: ACS Catalysis, Numéro 8/9, 2018, Page(s) 7734-7741, ISSN 2155-5435
Éditeur: American Chemical Society
DOI: 10.1021/acscatal.8b02208

CO Oxidation by N 2 O Homogeneously Catalyzed by Ruthenium Hydride Pincer Complexes Indicating a New Mechanism

Auteurs: Rong Zeng, Moran Feller, Yael Diskin-Posner, Linda J. W. Shimon, Yehoshoa Ben-David, David Milstein
Publié dans: Journal of the American Chemical Society, Numéro 140/23, 2018, Page(s) 7061-7064, ISSN 0002-7863
Éditeur: American Chemical Society
DOI: 10.1021/jacs.8b03927

Manganese-Catalyzed Direct Deoxygenation of Primary Alcohols

Auteurs: Jonathan O. Bauer, Subrata Chakraborty, David Milstein
Publié dans: ACS Catalysis, Numéro 7/7, 2017, Page(s) 4462-4466, ISSN 2155-5435
Éditeur: American Chemical Society
DOI: 10.1021/acscatal.7b01729

Template catalysis by manganese pincer complexes: oxa- and aza-Michael additions to unsaturated nitriles

Auteurs: Shan Tang, David Milstein
Publié dans: Chemical Science, 2019, ISSN 2041-6520
Éditeur: Royal Society of Chemistry
DOI: 10.1039/c9sc03269j

Ethylene glycol as an efficient and reversible liquid-organic hydrogen carrier

Auteurs: You-Quan Zou, Niklas von Wolff, Aviel Anaby, Yinjun Xie, David Milstein
Publié dans: Nature Catalysis, Numéro 2/5, 2019, Page(s) 415-422, ISSN 2520-1158
Éditeur: Springer Nature
DOI: 10.1038/s41929-019-0265-z

Facile synthesis of amides via acceptorless dehydrogenative coupling of aryl epoxides and amines

Auteurs: Yaoyu Liang, Jie Luo and David Milstein
Publié dans: Chemical Science, 2022, ISSN 2041-6520
Éditeur: Royal Society of Chemistry
DOI: 10.1039/d2sc01959k

Selective Hydrogenation of Nitriles to Secondary Imines Catalyzed by an Iron Pincer Complex

Auteurs: Subrata Chakraborty and David Milstein
Publié dans: ACS Catalysis, 2017, ISSN 2155-5435
Éditeur: American Chemical Society
DOI: 10.1021/acscatal.7b00906

Catalytic Hydrogenation of Thioesters, Thiocarbamates, and Thioamides

Auteurs: Jie Luo, Michael Rauch, Liat Avram, Yehoshoa Ben-David, David Milstein
Publié dans: Journal of the American Chemical Society, Numéro 142/52, 2020, Page(s) 21628-21633, ISSN 0002-7863
Éditeur: American Chemical Society
DOI: 10.1021/jacs.0c10884

Sustainable catalysis with fluxional acridine-based PNP pincer complexes

Auteurs: Sayan Kar and David Milstein
Publié dans: Chemical Communications, 2022, ISSN 1359-7345
Éditeur: Royal Society of Chemistry
DOI: 10.1039/d2cc00247g

Catalytic Furfural/5-Hydroxymethyl Furfural Oxidation to Furoic Acid/Furan-2,5-dicarboxylic Acid with H2 Production Using Alkaline Water as the Formal Oxidant

Auteurs: Sayan Kar; Quan-Quan Zhou; Yehoshoa Ben-David; David Milstein
Publié dans: Journal of the American Chemical Society, Numéro 1, 2022, ISSN 0002-7863
Éditeur: American Chemical Society
DOI: 10.1021/jacs.1c10908

Catalytic Oxidative Deamination by Water with H 2 Liberation

Auteurs: Shan Tang, Michael Rauch, Michael Montag, Yael Diskin-Posner, Yehoshoa Ben-David, David Milstein
Publié dans: Journal of the American Chemical Society, Numéro 142/49, 2020, Page(s) 20875-20882, ISSN 0002-7863
Éditeur: American Chemical Society
DOI: 10.1021/jacs.0c10826

Manganese Catalyzed Hydrogenation of Carbamates and Urea Derivatives

Auteurs: Uttam Kumar Das, Amit Kumar, Yehoshoa Ben-David, Mark A Iron and David Milstein
Publié dans: Journal of the American Chemical Society, 2019, ISSN 0002-7863
Éditeur: American Chemical Society
DOI: 10.1021/jacs.9b05591

Droits de propriété intellectuelle

MANGANESE BASED COMPLEXES AND USES THEREOF FOR HOMOGENEOUS CATALYSIS

Numéro de demande/publication: 20 708679
Date: 2017-02-08

REVERSIBLE LIQUID ORGANIC SYSTEM FOR LOADING AND DISCHARGING HYDROGEN BASED ON ETHYLENE GLYCOL

Numéro de demande/publication: 19 835832
Date: 2019-12-30

REVERSIBLE LIQUID ORGANIC SYSTEM, METHOD AND PROCESS FOR LOADING AND DISCHARGING HYDROGEN BASED ON N-HETEROCYCLES

Numéro de demande/publication: 20 708679
Date: 2020-02-06

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